Anisotropic Third-Harmonic Vortex Beam Generation with Ultrathin Germanium Arsenide Fork Gratings

Optical vortices have the tremendous potential to increase data capacity by leveraging the extra degree of freedom of orbital angular momentum. On the other hand, anisotropic 2D materials are promising building blocks for future integrated polarization-sensitive photonic and optoelectronic devices. Here, highly anisotropic third-harmonic optical vortex beam generation is demonstrated with fork holograms patterned on ultrathin 2D germanium arsenide flakes. It is shown that the anisotropic nonlinear vortex beam generation can be achieved independent of the fork grating orientation with respect to the crystallographic orientation. Furthermore, 2D fork hologram is designed to generate multiple optical vortices having different topological charges with strong anisotropic responses. These results pave the way toward the advancement of 2D material-based anisotropic nonlinear optical devices for future applications in photonic integrated circuits, optical communication, and optical information processing.