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Coherent Control of Internal Conversion in Strong-Field Molecular Ionization

  • Stony Brook University
  • Wigner Research Centre for Physics
  • Research Centre for Natural Sciences
  • University of Vienna

Research output: Contribution to journalArticlepeer-review

13 Scopus citations

Abstract

We demonstrate coherent control over internal conversion during strong-field molecular ionization with shaped, few-cycle laser pulses. The control is driven by interference in different neutral states, which are coupled via non-Born-Oppenheimer terms in the molecular Hamiltonian. Our measurements highlight the preservation of electronic coherence in nonadiabatic transitions between electronic states.

Original languageEnglish
Article number053202
JournalPhysical Review Letters
Volume125
Issue number5
DOIs
StatePublished - Jul 31 2020

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