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Electronic interactions in Dirac fluids visualized by nano-terahertz spacetime interference of electron-photon quasiparticles

  • Suheng Xu
  • , Yutao Li
  • , Rocco A. Vitalone
  • , Ran Jing
  • , Aaron J. Sternbach
  • , Shuai Zhang
  • , Julian Ingham
  • , Milan Delor
  • , James W. McIver
  • , Matthew Yankowitz
  • , Raquel Queiroz
  • , Andrew J. Millis
  • , Michael M. Fogler
  • , Cory R. Dean
  • , Abhay N. Pasupathy
  • , James Hone
  • , Mengkun Liu
  • , D. N. Basov
  • Columbia University
  • Brookhaven National Laboratory
  • Stony Brook University
  • Brookhaven National Laboratory Condensed Matter Physics and Materials Science Department
  • University of Maryland, College Park
  • University of Washington
  • Simons Foundation
  • University of California at San Diego

Research output: Contribution to journalArticlepeer-review

22 Scopus citations

Abstract

Ultraclean graphene at charge neutrality hosts a quantum critical Dirac fluid of interacting electrons and holes. Interactions profoundly affect the charge dynamics of graphene, which is encoded in the properties of its electron-photon collective modes: surface plasmon polaritons (SPPs). Here, we show that polaritonic interference patterns are particularly well suited to unveil the interactions in Dirac fluids by tracking polaritonic interference in time at temporal scales commensurate with the electronic scattering. Spacetime SPP interference patterns recorded in terahertz (THz) frequency range provided unobstructed readouts of the group velocity and lifetime of polariton that can be directly mapped onto the electronic spectral weight and the relaxation rate. Our data uncovered prominent departures of the electron dynamics from the predictions of the conventional Fermi-liquid theory. The deviations are particularly strong when the densities of electrons and holes are approximately equal. The proposed spacetime imaging methodology can be broadly applied to probe the electrodynamics of quantum materials.

Original languageEnglish
Article numbereado5553
JournalScience Advances
Volume10
Issue number43
DOIs
StatePublished - Oct 25 2024

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