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Interferometric measurements of the resonant nonlinearity of IR-active minor air constituents

  • J. J. Pigeon
  • , S. Y.A. Tochitsky
  • , D. Tovey
  • , G. J. Louwrens
  • , I. Ben-Zvi
  • , C. Joshi
  • Stony Brook University
  • University of California at Los Angeles

Research output: Contribution to journalArticlepeer-review

Abstract

The resonant nonlinear refractive indices of important IR-active, minor air constituents at mid-IR and long-wave IR wavelengths were measured using a Mach–Zehnder interferometer. Measurements in H2O vapor were performed near 2.94, 9.3, and 10.2 µm wavelengths, and measurements in CO2 and CO gas were performed near 9.3 µm. These measurements suggest that the nonlinearity of air can be greatly increased for relatively narrowband mid-IR and long-wave IR laser pulses.

Original languageEnglish
Pages (from-to)2878-2887
Number of pages10
JournalJournal of the Optical Society of America B: Optical Physics
Volume39
Issue number11
DOIs
StatePublished - Nov 2022

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