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Magnetic brightening and nanoscale imaging of spin-polarized helical edge modes in ZrTe5

  • Samuel Haeuser
  • , Richard H.J. Kim
  • , Lin Lin Wang
  • , Thomas Koschny
  • , Pedro M. Lozano
  • , Genda Gu
  • , Randall K. Chan
  • , Joong Mok Park
  • , Martin Mootz
  • , Liang Luo
  • , Qiang Li
  • , Jigang Wang
  • Ames Laboratory
  • Iowa State University
  • Brookhaven National Laboratory Condensed Matter Physics and Materials Science Department
  • Stony Brook University

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

Efficient charge transport remains a fundamental challenge for nanoelectronic devices, as their performance is constrained by high dissipation and the impedance mismatch between high-frequency signal sources and nanoscale circuit interfaces. Although topologically protected helical edge modes offer a dissipationless and backscattering-resilient alternative, achieving nanoscale control over these modes requires direct visualization of their spatial electrodynamics, especially under high-frequency operation. Here, by utilizing cryogenic magneto-infrared scattering-type scanning near-field optical microscopy (cm-IR-sSNOM), we image spin-polarized helical edge channels in ZrTe5 at the nanoscale, revealing magnetic-field-induced brightening as a high-frequency electrodynamic signature of robust topological edge modes. Operating at 1.8 K and under a magnetic field of up to 5 T, we observe the emergence of edge-state polarizability at infrared frequencies that is notably resilient to the magnetic gaps that typically quench d.c. and microwave edge transport. Our results reveal a topological ‘two-lane’ spatial reorganization in which an external magnetic field induces a spin-population imbalance between counterpropagating edge modes. Favoured helical branches are confined against physical boundaries to activate a net infrared near-field contrast. This electrodynamic response scales linearly with the number of atomic layers, which confirms that individual layers in ZrTe5 preserve their discrete quantum spin Hall identities. These findings may be useful for developing topological spintronic devices, as the magnetic infrared tunability of helical edge channels provides a pathway for low-loss nanoscale interconnects and high-speed information processing.

Original languageEnglish
Pages (from-to)1090-1096
Number of pages7
JournalNature Nanotechnology
Volume21
Issue number8
DOIs
StatePublished - Aug 2026

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