Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb

K. J. Gaffney; A. M. Lindenberg; J. Larsson; K. Sokolowski-Tinten; C. Blome; O. Synnergren; J. Sheppard; C. Caleman; A. G. MacPhee; D. Weinstein; D. P. Lowney; T. Allison; T. Matthews; R. W. Falcone; A. L. Cavalieri; D. M. Fritz; S. H. Lee; P. H. Bucksbaum; D. A. Reis; J. Rudati; A. T. MacRander; P. H. Fuoss; C. C. Kao; D. P. Siddons; R. Pahl; K. Moffat; J. Als-Nielsen; S. Duesterer; R. Ischebeck; H. Schlarb; H. Schulte-Schrepping; J. Schneider; D. Von Der Linde; O. Hignette; F. Sette; H. N. Chapman; R. W. Lee; T. N. Hansen; J. S. Wark; M. Bergh; G. Huldt; D. Van Der Spoel; N. Timneanu; J. Hajdu; R. A. Akre; E. Bong; P. Krejcik; J. Arthur; S. Brennan; K. Luening; J. B. Hastings

doi:10.1103/PhysRevLett.95.125701

Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb

K. J. Gaffney
, A. M. Lindenberg
, J. Larsson
, K. Sokolowski-Tinten
, C. Blome
, O. Synnergren
, J. Sheppard
, C. Caleman
, A. G. MacPhee
, D. Weinstein
, D. P. Lowney
, T. Allison
, T. Matthews
, R. W. Falcone
, A. L. Cavalieri
, D. M. Fritz
, S. H. Lee
, P. H. Bucksbaum
, D. A. Reis
, J. Rudati

A. T. MacRander, P. H. Fuoss, C. C. Kao, D. P. Siddons, R. Pahl, K. Moffat, J. Als-Nielsen, S. Duesterer, R. Ischebeck, H. Schlarb, H. Schulte-Schrepping, J. Schneider, D. Von Der Linde, O. Hignette, F. Sette, H. N. Chapman, R. W. Lee, T. N. Hansen, J. S. Wark, M. Bergh, G. Huldt, D. Van Der Spoel, N. Timneanu, J. Hajdu, R. A. Akre, E. Bong, P. Krejcik, J. Arthur, S. Brennan, K. Luening, J. B. Hastings

Chemistry

Stanford Synchrotron Radiation Lightsource
Lund University
Friedrich Schiller University Jena
University of Duisburg-Essen
German Electron Synchrotron
University of Oxford
Uppsala University
University of California at Berkeley
University of Michigan, Ann Arbor
Max Planck Institute of Quantum Optics
United States Department of Energy
Argonne National Laboratory
Brookhaven National Laboratory
The University of Chicago
University of Copenhagen
European Synchrotron Radiation Facility
Lawrence Livermore National Laboratory
SLAC National Accelerator Laboratory

Research output: Contribution to journal › Article › peer-review

53 Scopus citations

Abstract

The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.

Original language	English
Article number	125701
Journal	Physical Review Letters
Volume	95
Issue number	12
DOIs	https://doi.org/10.1103/PhysRevLett.95.125701
State	Published - Sep 16 2005

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Gaffney, K. J., Lindenberg, A. M., Larsson, J., Sokolowski-Tinten, K., Blome, C., Synnergren, O., Sheppard, J., Caleman, C., MacPhee, A. G., Weinstein, D., Lowney, D. P., Allison, T., Matthews, T., Falcone, R. W., Cavalieri, A. L., Fritz, D. M., Lee, S. H., Bucksbaum, P. H., Reis, D. A., ... Hastings, J. B. (2005). Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb. Physical Review Letters, 95(12), Article 125701. https://doi.org/10.1103/PhysRevLett.95.125701

@article{417712c8ba7747df929c4646c6811cde,

title = "Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb",

abstract = "The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.",

author = "Gaffney, \{K. J.\} and Lindenberg, \{A. M.\} and J. Larsson and K. Sokolowski-Tinten and C. Blome and O. Synnergren and J. Sheppard and C. Caleman and MacPhee, \{A. G.\} and D. Weinstein and Lowney, \{D. P.\} and T. Allison and T. Matthews and Falcone, \{R. W.\} and Cavalieri, \{A. L.\} and Fritz, \{D. M.\} and Lee, \{S. H.\} and Bucksbaum, \{P. H.\} and Reis, \{D. A.\} and J. Rudati and MacRander, \{A. T.\} and Fuoss, \{P. H.\} and Kao, \{C. C.\} and Siddons, \{D. P.\} and R. Pahl and K. Moffat and J. Als-Nielsen and S. Duesterer and R. Ischebeck and H. Schlarb and H. Schulte-Schrepping and J. Schneider and \{Von Der Linde\}, D. and O. Hignette and F. Sette and Chapman, \{H. N.\} and Lee, \{R. W.\} and Hansen, \{T. N.\} and Wark, \{J. S.\} and M. Bergh and G. Huldt and \{Van Der Spoel\}, D. and N. Timneanu and J. Hajdu and Akre, \{R. A.\} and E. Bong and P. Krejcik and J. Arthur and S. Brennan and K. Luening and Hastings, \{J. B.\}",

year = "2005",

month = sep,

day = "16",

doi = "10.1103/PhysRevLett.95.125701",

language = "English",

volume = "95",

journal = "Physical Review Letters",

issn = "0031-9007",

number = "12",

}

Gaffney, KJ, Lindenberg, AM, Larsson, J, Sokolowski-Tinten, K, Blome, C, Synnergren, O, Sheppard, J, Caleman, C, MacPhee, AG, Weinstein, D, Lowney, DP, Allison, T, Matthews, T, Falcone, RW, Cavalieri, AL, Fritz, DM, Lee, SH, Bucksbaum, PH, Reis, DA, Rudati, J, MacRander, AT, Fuoss, PH, Kao, CC, Siddons, DP, Pahl, R, Moffat, K, Als-Nielsen, J, Duesterer, S, Ischebeck, R, Schlarb, H, Schulte-Schrepping, H, Schneider, J, Von Der Linde, D, Hignette, O, Sette, F, Chapman, HN, Lee, RW, Hansen, TN, Wark, JS, Bergh, M, Huldt, G, Van Der Spoel, D, Timneanu, N, Hajdu, J, Akre, RA, Bong, E, Krejcik, P, Arthur, J, Brennan, S, Luening, K & Hastings, JB 2005, 'Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb', Physical Review Letters, vol. 95, no. 12, 125701. https://doi.org/10.1103/PhysRevLett.95.125701

TY - JOUR

T1 - Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb

AU - Gaffney, K. J.

AU - Lindenberg, A. M.

AU - Larsson, J.

AU - Sokolowski-Tinten, K.

AU - Blome, C.

AU - Synnergren, O.

AU - Sheppard, J.

AU - Caleman, C.

AU - MacPhee, A. G.

AU - Weinstein, D.

AU - Lowney, D. P.

AU - Allison, T.

AU - Matthews, T.

AU - Falcone, R. W.

AU - Cavalieri, A. L.

AU - Fritz, D. M.

AU - Lee, S. H.

AU - Bucksbaum, P. H.

AU - Reis, D. A.

AU - Rudati, J.

AU - MacRander, A. T.

AU - Fuoss, P. H.

AU - Kao, C. C.

AU - Siddons, D. P.

AU - Pahl, R.

AU - Moffat, K.

AU - Als-Nielsen, J.

AU - Duesterer, S.

AU - Ischebeck, R.

AU - Schlarb, H.

AU - Schulte-Schrepping, H.

AU - Schneider, J.

AU - Von Der Linde, D.

AU - Hignette, O.

AU - Sette, F.

AU - Chapman, H. N.

AU - Lee, R. W.

AU - Hansen, T. N.

AU - Wark, J. S.

AU - Bergh, M.

AU - Huldt, G.

AU - Van Der Spoel, D.

AU - Timneanu, N.

AU - Hajdu, J.

AU - Akre, R. A.

AU - Bong, E.

AU - Krejcik, P.

AU - Arthur, J.

AU - Brennan, S.

AU - Luening, K.

AU - Hastings, J. B.

PY - 2005/9/16

Y1 - 2005/9/16

N2 - The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.

AB - The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.

UR - https://www.scopus.com/pages/publications/27144512107

U2 - 10.1103/PhysRevLett.95.125701

DO - 10.1103/PhysRevLett.95.125701

M3 - Article

AN - SCOPUS:27144512107

SN - 0031-9007

VL - 95

JO - Physical Review Letters

JF - Physical Review Letters

IS - 12

M1 - 125701

ER -

Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb

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