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Rapid simulations of hyperspectral near-field images of three-dimensional heterogeneous surfaces - part II

  • Xinzhong Chen
  • , Ziheng Yao
  • , Zhiyuan Sun
  • , Stefan G. Stanciu
  • , D. N. Basov
  • , Rainer Hillenbrand
  • , Mengkun Liu
  • Stony Brook University
  • Harvard University
  • National University of Science and Technology POLITEHNICA Bucharest
  • Columbia University
  • CIC nanoGUNE
  • Ikerbasque Basque Foundation for Science

Research output: Contribution to journalArticlepeer-review

27 Scopus citations

Abstract

The modeling of the near-field interaction in the scattering-type scanning near-field optical microscope (s-SNOM) is rapidly advancing, although an accurate yet versatile modeling framework that can be easily adapted to various complex situations is still lacking. In this work, we propose a time-efficient numerical scheme in the quasi-electrostatic limit to capture the tip-sample interaction in the near field. This method considers an extended tip geometry, which is a significant advantage compared to the previously reported method based on the point-dipole approximation. Using this formalism, we investigate, among others, nontrivial questions such as uniaxial and biaxial anisotropy in the near-field interaction, the relationship between various experimental parameters (e.g. tip radius, tapping amplitude, etc.), and the tip-dependent spatial resolution. The demonstrated method further sheds light on the understanding of the contrast mechanism in s-SNOM imaging and spectroscopy, while also representing a valuable platform for future quantitative analysis of the experimental observations.

Original languageEnglish
Pages (from-to)11228-11242
Number of pages15
JournalOptics Express
Volume30
Issue number7
DOIs
StatePublished - Mar 28 2022

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