Toward strong field mode-selective chemistry

T. C. Weinacht; J. L. White; P. H. Bucksbaum

doi:10.1021/jp991977x

Toward strong field mode-selective chemistry

T. C. Weinacht
, J. L. White
, P. H. Bucksbaum

Physics and Astronomy

University of Michigan, Ann Arbor

Research output: Contribution to journal › Article › peer-review

164 Scopus citations

Abstract

We demonstrate a new method for coherent control of bond excitation in the strong field regime. We can selectively excite one or more Raman-active modes in a molecular liquid without the need for externally generated coherent sources separated by the Stokes frequency. The method employs excitation with an intense phase-shaped pulse in a learning control loop.

Original language	English
Pages (from-to)	10166-10168
Number of pages	3
Journal	Journal of Physical Chemistry A
Volume	103
Issue number	49
DOIs	https://doi.org/10.1021/jp991977x
State	Published - Dec 9 1999

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title = "Toward strong field mode-selective chemistry",

abstract = "We demonstrate a new method for coherent control of bond excitation in the strong field regime. We can selectively excite one or more Raman-active modes in a molecular liquid without the need for externally generated coherent sources separated by the Stokes frequency. The method employs excitation with an intense phase-shaped pulse in a learning control loop.",

author = "Weinacht, \{T. C.\} and White, \{J. L.\} and Bucksbaum, \{P. H.\}",

year = "1999",

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language = "English",

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T1 - Toward strong field mode-selective chemistry

AU - Weinacht, T. C.

AU - White, J. L.

AU - Bucksbaum, P. H.

PY - 1999/12/9

Y1 - 1999/12/9

N2 - We demonstrate a new method for coherent control of bond excitation in the strong field regime. We can selectively excite one or more Raman-active modes in a molecular liquid without the need for externally generated coherent sources separated by the Stokes frequency. The method employs excitation with an intense phase-shaped pulse in a learning control loop.

AB - We demonstrate a new method for coherent control of bond excitation in the strong field regime. We can selectively excite one or more Raman-active modes in a molecular liquid without the need for externally generated coherent sources separated by the Stokes frequency. The method employs excitation with an intense phase-shaped pulse in a learning control loop.

UR - https://www.scopus.com/pages/publications/0001630526

U2 - 10.1021/jp991977x

DO - 10.1021/jp991977x

M3 - Article

AN - SCOPUS:0001630526

SN - 1089-5639

VL - 103

SP - 10166

EP - 10168

JO - Journal of Physical Chemistry A

JF - Journal of Physical Chemistry A

IS - 49

ER -

Toward strong field mode-selective chemistry

Abstract

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